How add Album with my songs?
I tried add mp3 tag with Album, but useless.
Could some one help?
The albums are based on the album tags in your audio files. However, if you just added those tags, then they probably only show up after the next sync.
As to how to add the album information: there are a lot of programs available that can do that for you. Windows Explorer can do it, although it's not that practical for large batches. mp3tag is a popular choice for batch tag editing on Windows (just don't forget to save like I tend to do). iTunes can do it too.
If you want to automatically find the (mostly) correct tags for your songs, it might also be worth looking at MusicBrainz Picard.